By Stuart A. Rice
The Advances in Chemical Physics sequence offers the innovative in each zone of the self-discipline and offers the sphere with a discussion board for serious, authoritative reviews of advances. It presents an article framework that makes the ebook an outstanding complement to complex graduate sessions, with contributions from specialists all over the world and a convenient thesaurus for simple reference on new terminology. This sequence is an excellent advisor for college students and pros in chemical physics and actual chemistry, from academia, executive, and industries together with chemical substances, prescribed drugs, and polymers.
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Extra resources for Advances in Chemical Physics, Vol. 141
In the first one, the control fields are constructed employing information on the entire dynamics from time ti to time tf , whereas in a local control scheme, the field is determined instantaneously, taking the system’s response into account. For a review on early work on local optimization, see Ref. 41. In this chapter we review our recent applications of a local control scheme to various problems in chemical physics. The approach we follow is called Local Control Theory (LCT). The idea first appeared in the formulation of Optimal Control Theory introduced by Kosloff, Rice, and Tannor  and has been local control theory 31 extensively developed since then [41,43–51].
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Dissociation and predissociation dynamics in a cooling field. , as indicated. The predissociation yield B0 ðtÞ is shown in the upper panel, which also contains the field free case. To conclude this subsection, we demonstrated that heating and cooling LCT fields can be employed to modify the branching ratio of ground-state predissociation and excited-state dissociation. Furthermore, a stabilization of predissociating molecules can temporarily be maintained. C. Photodissociation via Selective Mode Excitation The last subsections treated an example of a diatomic molecule where a single degree of freedom is present.
Advances in Chemical Physics, Vol. 141 by Stuart A. Rice